We inquired about this earlier, and were told that it couldn't be done with Chrome.
Chrome extension - pre-configure sites list
We have successfully deployed the ND extension for the Chrome browser. It would however be really useful if we could deploy a default list of connected sites to our users. It would reduce the need to train this feature as we could automatically set up connections to sites where users commonly upload/download documents.
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It is kind of round-about but I think you can if you deploy them via registry keys:
Provided you have a demo machine to set it up from beforehand.
Does the Chrome extension allow you to preview what you are uploading/downloading before saving to the workspace?